| 1. Ray Anthony, Ken Jones; Walter Schumann - Dragnet/Room 43 | not rated | 4:54 |
| 2. Earle H. Hagen, Earle H. Hagen - I Spy | not rated | 2:12 |
| 3. Elmer Bernstein, Elmer Bernstein - Thinking of Baby | not rated | 3:03 |
| 4. Count Basie, Lionel Bart - From Russia With Love | not rated | 4:16 |
| 5. Laurindo Almeida, Laurindo Almeida - Big Town | not rated | 2:44 |
| 6. Billy May, Elmer Bernstein; Sylvia Fine - Man With the Golden Arm | not rated | 2:51 |
| 7. Nelson Riddle, Nelson Riddle - The Untouchables | not rated | 2:19 |
| 8. Leroy Hadidi, Monty Norman - The James Bond Theme | not rated | 4:35 |
| 9. Billy May, Lalo Schifrin - Mission: Impossible | not rated | 2:27 |
| 10. Spike Jones' New Band, Earle H. Hagen - Harlem Nocturne | not rated | 2:27 |
| 11. Si Zentner, Elmer Bernstein; Mack David - Walk on the Wild Side | not rated | 2:36 |
| 12. Elliott Fisher, John Barry; Leslie Bricusse - Mr. Kiss Kiss Bang Bang | not rated | 1:52 |
| 13. Lou Busch, Leon Pober - The Wild Ones | not rated | 2:28 |
| 14. Elmer Bernstein, Elmer Bernstein - Staccato's Theme | not rated | 2:55 |
| 15. Leroy Hadidi, John Barry - Search for Vulcan | not rated | 2:52 |
| 16. Ray Anthony, Henry Mancini - Peter Gunn Suite: Walkin' to Mother's/Fall Out/Dreamsville/Peter Gunn | not rated | 8:33 |
| 17. Vikki Carr, David M.; Elmer Bernstein - The Silences | not rated | 2:57 |
| 18. Alfred Hitchcock; Jeff Alexander, Jeff Alexander - Music to Be Murdered By | not rated | 5:00 |
| 19. Renzo Cesana - Walk the Lonesome Night | not rated | 2:29 |
| 1:03:30 |
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